Publication Date
12-18-2025
Document Type
Article
Publication Title
ACS Omega
Volume
11
Issue
1
DOI
10.1021/acsomega.5c07669
First Page
1012
Last Page
1018
Abstract
The coin cell form factor has become a standard in energy storage research owing to its relatively low cost, low quantity of requisite electroactive material, fast experimental turnover, and capability to generate publishable quality data. Coin cell assembly at the lab-scale requires precise manual alignment of the many internal components of a cell to yield a properly functioning device. Truly repeatable device assembly presents a significant challenge to the acquisition of reliable data. In this report, we present a three-dimensional (3D) printable design for a coin cell alignment device and describe techniques for a generalized workflow to achieve reproducible coin cell assembly of lithium-based batteries. Standardized assembly techniques using readily accessible, purpose-built tools were demonstrated for lab-scale production of lithium–sulfur (Li–S) coin cells. Li–S batteries fabricated using the alignment device as well as conductive adhesive incorporated workflows afforded coin cells with up to 35% reduction of assembly times, comparable or better functional cell yields, and improved electrochemical device performance with more consistent and up to 150 mAh/g higher average discharge capacities coupled with Coulombic efficiency increases of up to 2.0% over manually aligned cell assembly techniques.
Funding Number
DE-SC0024581
Funding Sponsor
U.S. Department of Energy
Creative Commons License

This work is licensed under a Creative Commons Attribution-Noncommercial-No Derivative Works 4.0 License.
Department
Chemistry
Recommended Citation
Daryl Miranda, Tosif Aliyev, Lamija Kovacevic, Sivapriya Voleti, Jaydie Lee, Kathleen Meehan, Monica C. So, and Philip T. Dirlam. "Lithium–Sulfur Batteries: 3D Printed Tools and Assembly Techniques for Repeatable Lab-Scale Coin Cell Manufacturing" ACS Omega (2025): 1012-1018. https://doi.org/10.1021/acsomega.5c07669